TY - JOUR

T1 - Causality and quantum interference in time-delayed laser-induced nonsequential double ionization

AU - Shaaran, Tahir

AU - Figueira de Morisson Faria, C.

AU - Schomerus, Henning

N1 - ©2012 American Physical Society

PY - 2012/2/23

Y1 - 2012/2/23

N2 - We perform a detailed analysis of the importance of causality within the strong-field approximation and the steepest-descent framework for the recollision-excitation with subsequent tunneling ionization (RESI) pathway in laser-induced nonsequential double ionization (NSDI). In this time-delayed pathway, an electron returns to its parent ion and, by recolliding with the core, gives part of its kinetic energy to excite a second electron at a time t′. The second electron then reaches the continuum at a later time t by tunneling ionization. We show that, if t′ and t are complex, the condition that recollision of the first electron occurs before tunnel ionization of the second electron translates into boundary conditions for the steepest-descent contours and thus puts constraints on the saddles to be taken when computing the RESI transition amplitudes. We also show that this generalized causality condition has a dramatic effect on the shapes of the RESI electron momentum distributions for few-cycle laser pulses. Physically, causality determines how the dominant sets of orbits of an electron returning to its parent ion can be combined with the dominant orbits of a second electron tunneling from an excited state. All features encountered are analyzed in terms of such orbits and their quantum interference.

AB - We perform a detailed analysis of the importance of causality within the strong-field approximation and the steepest-descent framework for the recollision-excitation with subsequent tunneling ionization (RESI) pathway in laser-induced nonsequential double ionization (NSDI). In this time-delayed pathway, an electron returns to its parent ion and, by recolliding with the core, gives part of its kinetic energy to excite a second electron at a time t′. The second electron then reaches the continuum at a later time t by tunneling ionization. We show that, if t′ and t are complex, the condition that recollision of the first electron occurs before tunnel ionization of the second electron translates into boundary conditions for the steepest-descent contours and thus puts constraints on the saddles to be taken when computing the RESI transition amplitudes. We also show that this generalized causality condition has a dramatic effect on the shapes of the RESI electron momentum distributions for few-cycle laser pulses. Physically, causality determines how the dominant sets of orbits of an electron returning to its parent ion can be combined with the dominant orbits of a second electron tunneling from an excited state. All features encountered are analyzed in terms of such orbits and their quantum interference.

U2 - 10.1103/PhysRevA.85.023423

DO - 10.1103/PhysRevA.85.023423

M3 - Journal article

VL - 85

JO - Physical review a

JF - Physical review a

SN - 1050-2947

IS - 2

M1 - 023423

ER -