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Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model

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Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model. / Touitou, Jamal; Aiouache, Farid; Burch, Robbie et al.
In: Journal of Catalysis, Vol. 319, 11.2014, p. 239-246.

Research output: Contribution to Journal/Magazine › Journal article › peer-review

Harvard

Touitou, J, Aiouache, F, Burch, R, Roy, D, Hardacre, C, Morgan, K, Sa, J, Stewart, C, Stewart, J & Goguet, A 2014, 'Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model', Journal of Catalysis, vol. 319, pp. 239-246. https://doi.org/10.1016/j.jcat.2014.09.006

APA

Touitou, J., Aiouache, F., Burch, R., Roy, D., Hardacre, C., Morgan, K., Sa, J., Stewart, C., Stewart, J., & Goguet, A. (2014). Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model. Journal of Catalysis, 319, 239-246. https://doi.org/10.1016/j.jcat.2014.09.006

Vancouver

Touitou J, Aiouache F, Burch R, Roy D, Hardacre C, Morgan K et al. Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model. Journal of Catalysis. 2014 Nov;319:239-246. Epub 2014 Oct 3. doi: 10.1016/j.jcat.2014.09.006

Author

Touitou, Jamal ; Aiouache, Farid ; Burch, Robbie et al. / Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model. In: Journal of Catalysis. 2014 ; Vol. 319. pp. 239-246.

Bibtex

@article{53ac116bead34eaea827d4ef365781ab,
title = "Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model",
abstract = "This paper reports the detailed description and validation of a fully automated, computer controlled analytical method to spatially probe the gas composition and thermal characteristics in packed bed systems. This method has been designed to limit the invasiveness of the probe, a characteristic assessed using CFD. The thermocouple is aligned with the sampling holes to enable simultaneous recording of the gas composition and temperature profiles. This analysis technique has been validated by studying CO oxidation over a 1% Pt/Al2O3 catalyst. The resultant profiles have been compared with a micro-kinetic model, to further assess the strength of the technique.",
keywords = "Spatially resolved profiles, Micro-kinetic model, Comutational fluid dynamics",
author = "Jamal Touitou and Farid Aiouache and Robbie Burch and Douglas Roy and Christopher Hardacre and Kevin Morgan and Jacinto Sa and Caomhan Stewart and Jonathan Stewart and Alexandre Goguet",
year = "2014",
month = nov,
doi = "10.1016/j.jcat.2014.09.006",
language = "English",
volume = "319",
pages = "239--246",
journal = "Journal of Catalysis",
issn = "0021-9517",
publisher = "Academic Press Inc.",

}

RIS

TY - JOUR

T1 - Evaluation of an in situ spatial resolution instrument for fixed beds through the assessment of the invasiveness of probes and a comparison with a micro-kinetic model

AU - Touitou, Jamal

AU - Aiouache, Farid

AU - Burch, Robbie

AU - Roy, Douglas

AU - Hardacre, Christopher

AU - Morgan, Kevin

AU - Sa, Jacinto

AU - Stewart, Caomhan

AU - Stewart, Jonathan

AU - Goguet, Alexandre

PY - 2014/11

Y1 - 2014/11

N2 - This paper reports the detailed description and validation of a fully automated, computer controlled analytical method to spatially probe the gas composition and thermal characteristics in packed bed systems. This method has been designed to limit the invasiveness of the probe, a characteristic assessed using CFD. The thermocouple is aligned with the sampling holes to enable simultaneous recording of the gas composition and temperature profiles. This analysis technique has been validated by studying CO oxidation over a 1% Pt/Al2O3 catalyst. The resultant profiles have been compared with a micro-kinetic model, to further assess the strength of the technique.

AB - This paper reports the detailed description and validation of a fully automated, computer controlled analytical method to spatially probe the gas composition and thermal characteristics in packed bed systems. This method has been designed to limit the invasiveness of the probe, a characteristic assessed using CFD. The thermocouple is aligned with the sampling holes to enable simultaneous recording of the gas composition and temperature profiles. This analysis technique has been validated by studying CO oxidation over a 1% Pt/Al2O3 catalyst. The resultant profiles have been compared with a micro-kinetic model, to further assess the strength of the technique.

KW - Spatially resolved profiles

KW - Micro-kinetic model

KW - Comutational fluid dynamics

U2 - 10.1016/j.jcat.2014.09.006

DO - 10.1016/j.jcat.2014.09.006

M3 - Journal article

VL - 319

SP - 239

EP - 246

JO - Journal of Catalysis

JF - Journal of Catalysis

SN - 0021-9517

ER -