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    Rights statement: This is the peer reviewed version of the following articleJ. Zou, A. Trewin, T. Ben, S. Qiu, Angew. Chem. Int. Ed. 2020, 59, 769 which has been published in final form at https://onlinelibrary.wiley.com/doi/10.1002/anie.201913380 This article may be used for non-commercial purposes in accordance With Wiley Terms and Conditions for self-archiving.

    Accepted author manuscript, 1.38 MB, PDF document

    Embargo ends: 2/12/20

    Available under license: CC BY-NC: Creative Commons Attribution-NonCommercial 4.0 International License

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High Uptake and Fast Transportation of LiPF6 in a Porous Aromatic Framework for Solid-State Li-Ion Batteries

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<mark>Journal publication date</mark>7/01/2020
<mark>Journal</mark>Angewandte Chemie - International Edition
Issue number2
Volume59
Number of pages6
Pages (from-to)769-774
Publication StatusPublished
Early online date2/12/19
<mark>Original language</mark>English

Abstract

Solid-state Li-ion batteries (SSLIBs) have recently attracted substantial attention from scientists for the advantages of better safety performance. However, there are still several key challenges in SSLIBs that need to be addressed, such as low energy density, poor thermal stability or cycle stability, and large interface resistance. This contribution introduces a novel SSLIB with a porous aromatic framework (PAF-1) accommodating LiPF6 that was used as the solid-state electrolyte (SSE) replacing the liquid electrolyte and diaphragm of traditional Li-ion batteries. The charge, discharge capacity, rate performance and cycle stability of the SSLIB were remarkably enhanced.

Bibliographic note

This is the peer reviewed version of the following articleJ. Zou, A. Trewin, T. Ben, S. Qiu, Angew. Chem. Int. Ed. 2020, 59, 769 which has been published in final form at https://onlinelibrary.wiley.com/doi/10.1002/anie.201913380 This article may be used for non-commercial purposes in accordance With Wiley Terms and Conditions for self-archiving.