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Giant thermopower and figure of merit in single-molecule devices

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Giant thermopower and figure of merit in single-molecule devices. / Finch, C. M.; Garcia-Suarez, V. M.; Lambert, Colin.
In: Physical review B, Vol. 79, No. 3, 033405, 01.2009, p. -.

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Finch CM, Garcia-Suarez VM, Lambert C. Giant thermopower and figure of merit in single-molecule devices. Physical review B. 2009 Jan;79(3):-. 033405. doi: 10.1103/PhysRevB.79.033405

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Finch, C. M. ; Garcia-Suarez, V. M. ; Lambert, Colin. / Giant thermopower and figure of merit in single-molecule devices. In: Physical review B. 2009 ; Vol. 79, No. 3. pp. -.

Bibtex

@article{00d4a22de9284780843768795cc7b6dc,
title = "Giant thermopower and figure of merit in single-molecule devices",
abstract = "We present a study of the thermopower S and the dimensionless figure of merit ZT in molecules sandwiched between gold electrodes. We show that for molecules with side groups, the shape of the transmission coefficient can be dramatically modified by Fano resonances near the Fermi energy, which can be tuned to produce huge increases in S and ZT. This shows that molecules exhibiting Fano resonances have a high efficiency of thermoelectric cooling which is not present for conventional ungated molecules with only delocalized states along their backbone.",
author = "Finch, {C. M.} and Garcia-Suarez, {V. M.} and Colin Lambert",
year = "2009",
month = jan,
doi = "10.1103/PhysRevB.79.033405",
language = "English",
volume = "79",
pages = "--",
journal = "Physical review B",
issn = "1098-0121",
publisher = "AMER PHYSICAL SOC",
number = "3",

}

RIS

TY - JOUR

T1 - Giant thermopower and figure of merit in single-molecule devices

AU - Finch, C. M.

AU - Garcia-Suarez, V. M.

AU - Lambert, Colin

PY - 2009/1

Y1 - 2009/1

N2 - We present a study of the thermopower S and the dimensionless figure of merit ZT in molecules sandwiched between gold electrodes. We show that for molecules with side groups, the shape of the transmission coefficient can be dramatically modified by Fano resonances near the Fermi energy, which can be tuned to produce huge increases in S and ZT. This shows that molecules exhibiting Fano resonances have a high efficiency of thermoelectric cooling which is not present for conventional ungated molecules with only delocalized states along their backbone.

AB - We present a study of the thermopower S and the dimensionless figure of merit ZT in molecules sandwiched between gold electrodes. We show that for molecules with side groups, the shape of the transmission coefficient can be dramatically modified by Fano resonances near the Fermi energy, which can be tuned to produce huge increases in S and ZT. This shows that molecules exhibiting Fano resonances have a high efficiency of thermoelectric cooling which is not present for conventional ungated molecules with only delocalized states along their backbone.

UR - http://www.scopus.com/inward/record.url?scp=59249090719&partnerID=8YFLogxK

U2 - 10.1103/PhysRevB.79.033405

DO - 10.1103/PhysRevB.79.033405

M3 - Journal article

VL - 79

SP - -

JO - Physical review B

JF - Physical review B

SN - 1098-0121

IS - 3

M1 - 033405

ER -