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Deactivation of the preferential oxidation of CO in packed bed reactor by 3D modelling and near-infrared tomography

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mov1. Axial sectional map of concentration of H2OV, time-on-stream of 60 min, respectively, PBR of an AR of 13— i.e., particle size of 0.9 mm, feed temperature of 413 K, flow rate of 670 cm3 min−1, and composition: 1.1 mol % at steady-state and increased to 1.4% CO at transient conditions, 2.5 mol% O2, 1.7 mol % H2 and N2 as carrier gas.
mov2. 3D views and cross-sectional map of activity at time-on-stream of 120 min, cross-section at 15mm from the inlet of the PBR, PBR of 10mm ID, 25mm length, particle size of 1 mm, feed flow rate of 470 cm3 min−1 and composition: 1.1 mol% at steady-state and increased to 1.4 mol% CO at transient conditions along with deactivation, 1.7 mol% H2 and N2 as carrier gas.
mov3. Cross-sectional map of activity at time-on-stream of 120 min, cross-section at 15mm from the inlet of the PBR, PBR of 10mm ID, 25mm length, particle size of 1 mm, feed flow rate of 470 cm3 min−1 and composition: 1.1 mol% at steady-state and increased to 1.4 mol% CO at transient conditions along with deactivation, 1.7 mol% H2 and N2 as carrier gas.
Date made available2019
PublisherLancaster University

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