TY - JOUR

T1 - Aircraft study of Mountain Chimney Effect of Beijing, China

AU - Chen, Ying

AU - Zhao, Chunsheng

AU - Zhang, Qiang

AU - Deng, Zhaoze

AU - Huang, Mengyu

AU - Ma, Xincheng

N1 - D08306

PY - 2009/4/27

Y1 - 2009/4/27

N2 - [1] In this paper, the three-dimensional distribution of air pollutants in the Beijing region using aircraft measurements is reported, and Mountain Chimney Effect (MCE) on the distribution of air pollutants in this region is studied. A remarkable two-pollution-layer structure was observed by aircraft measurement in Beijing on 18 August 2007. Gaseous and particle pollutants were well mixed with high concentrations in the planetary boundary layer. There was an elevated pollution layer (EPL) at the altitude of 2500–3500 m, and the concentrations of pollutants were high and comparable with that in the planetary boundary layer. Analysis of aircraft measurement indicates that pollutants in the two pollution layers originated from the same source. On the basis of analysis of the Weather Research and Forecasting (WRF)-TRACER model and wind profile data, the formation of EPL is discussed. The wind flow of Beijing region was dominated by mountain-valley breeze, which has MCE on the distribution of pollutants in this region. Air pollutants were injected from the planetary boundary layer into the free troposphere due to this effect. These pollutants were subsequently transported back over the city by the elevated northerly wind. Thus the structure of two pollution layers over Beijing is formed. Modeling results show that the persistence of a polluted layer over the boundary layer from the previous day has significant contribution to the surface concentrations of pollutants. When the mixing depth increases, the elevated pollutants are recaptured into planetary boundary layer and mixed downward. The rapid increase of surface concentrations of pollutants may be attributed to the vertical down-mixing of pollutants.

AB - [1] In this paper, the three-dimensional distribution of air pollutants in the Beijing region using aircraft measurements is reported, and Mountain Chimney Effect (MCE) on the distribution of air pollutants in this region is studied. A remarkable two-pollution-layer structure was observed by aircraft measurement in Beijing on 18 August 2007. Gaseous and particle pollutants were well mixed with high concentrations in the planetary boundary layer. There was an elevated pollution layer (EPL) at the altitude of 2500–3500 m, and the concentrations of pollutants were high and comparable with that in the planetary boundary layer. Analysis of aircraft measurement indicates that pollutants in the two pollution layers originated from the same source. On the basis of analysis of the Weather Research and Forecasting (WRF)-TRACER model and wind profile data, the formation of EPL is discussed. The wind flow of Beijing region was dominated by mountain-valley breeze, which has MCE on the distribution of pollutants in this region. Air pollutants were injected from the planetary boundary layer into the free troposphere due to this effect. These pollutants were subsequently transported back over the city by the elevated northerly wind. Thus the structure of two pollution layers over Beijing is formed. Modeling results show that the persistence of a polluted layer over the boundary layer from the previous day has significant contribution to the surface concentrations of pollutants. When the mixing depth increases, the elevated pollutants are recaptured into planetary boundary layer and mixed downward. The rapid increase of surface concentrations of pollutants may be attributed to the vertical down-mixing of pollutants.

KW - Pollution: urban and regional, Troposphere: composition and chemistry, Troposphere: constituent transport and chemistry, mountain-valley breezes, Mountain Chimney Effect, Beijing, aircraft, ozone, aerosol

U2 - 10.1029/2008JD010610

DO - 10.1029/2008JD010610

M3 - Journal article

VL - 114

JO - Journal of Geophysical Research

JF - Journal of Geophysical Research

SN - 2156-2202

IS - D8

ER -