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High-Resolution Convective Wet Scavenging Simulations: A Case Study of the Fukushima Daiichi Nuclear Power Plant Accident

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E-pub ahead of print
  • Nuohang Liu
  • Baozhu Ge
  • Xingtao Su
  • Xueshun Chen
  • Oliver Wild
  • Yuanchun Zhang
  • Zhe Wang
  • Zifa Wang
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Article numbere2024JD043202
<mark>Journal publication date</mark>28/08/2025
<mark>Journal</mark>Journal of Geophysical Research: Atmospheres
Issue number16
Volume130
Number of pages19
Publication StatusE-pub ahead of print
Early online date20/08/25
<mark>Original language</mark>English

Abstract

Abstract Convective precipitation is a key factor for diagnosing convective clouds and the subsequent modeling of the wet scavenging of air pollutants in offline chemical transport models (CTMs). However, a discrepancy exists between the Weather Research and Forecasting model, which uses resolved convection, and CTMs, which rely on a diagnostic convective cloud scheme, in handling high-resolution convective wet scavenging simulations. To explore the uncertainties arising from this disparity, this study focuses on 137Cs, released during the Fukushima Daiichi Nuclear Power Plant accident, as a species with numerous observations compared to other radionuclides and minimal interference from other factors using the NAQPMS model incorporating a physically-based wet deposition module. A diagnostic convective cloud scheme was applied, using a radar composite reflectivity factor (RCRF) of 35 dBZ to identify convective precipitation. Implementing the RCRF diagnosis scheme significantly improved model performance by increasing in-cloud deposition. This enhancement led to a 4648resolution convective wet scavenging using offline CTMs.

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e2024JD043202 2024JD043202