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Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation

Research output: Contribution to Journal/Magazine › Journal article › peer-review

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Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation. / Plant, Arran; Kos, Bor; Jazbec, Anze et al.
In: Industrial and Engineering Chemistry Research, Vol. 62, No. 49, 13.12.2023, p. 21152-21163.

Research output: Contribution to Journal/Magazine › Journal article › peer-review

Harvard

Plant, A, Kos, B, Jazbec, A, Snoj, L, Joyce, M & Najdanovic‐Visak, V 2023, 'Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation', Industrial and Engineering Chemistry Research, vol. 62, no. 49, pp. 21152-21163. https://doi.org/10.1021/acs.iecr.3c03317

APA

Plant, A., Kos, B., Jazbec, A., Snoj, L., Joyce, M., & Najdanovic‐Visak, V. (2023). Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation. Industrial and Engineering Chemistry Research, 62(49), 21152-21163. https://doi.org/10.1021/acs.iecr.3c03317

Vancouver

Plant A, Kos B, Jazbec A, Snoj L, Joyce M, Najdanovic‐Visak V. Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation. Industrial and Engineering Chemistry Research. 2023 Dec 13;62(49):21152-21163. Epub 2023 Dec 4. doi: 10.1021/acs.iecr.3c03317

Author

Plant, Arran ; Kos, Bor ; Jazbec, Anze et al. / Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation. In: Industrial and Engineering Chemistry Research. 2023 ; Vol. 62, No. 49. pp. 21152-21163.

Bibtex

@article{105b9fd7a8ce4505bbfdfaab9568522a,
title = "Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation",
abstract = "Despite offering low-carbon and reliable energy, the utilization of nuclear energy is declining globally due to high upfront capital costs and longer returns on investments. Nuclear cogeneration of valuable chemicals from waste biomass-derived feedstocks could have beneficial impacts while harnessing the underutilized resource of ionizing energy. Here, we demonstrate selective methanol or acetaldehyde production from ethylene glycol, a feedstock derived from glycerol, a byproduct of biodiesel, using irradiations from a nuclear fission reactor. The influence of radiation quality, dose rate, and the absorbed dose of irradiations on radiochemical yields (G-value) has been studied. Under low-dose-rate, γ-only radiolysis during reactor shutdown rate (",
author = "Arran Plant and Bor Kos and Anze Jazbec and Luca Snoj and Malcolm Joyce and Vesna Najdanovic‐Visak",
year = "2023",
month = dec,
day = "13",
doi = "10.1021/acs.iecr.3c03317",
language = "English",
volume = "62",
pages = "21152--21163",
journal = "Industrial and Engineering Chemistry Research",
issn = "0888-5885",
publisher = "American Chemical Society",
number = "49",

}

RIS

TY - JOUR

T1 - Nuclear Cogeneration of Methanol and Acetaldehyde from Ethylene Glycol Using Ionizing Radiation

AU - Plant, Arran

AU - Kos, Bor

AU - Jazbec, Anze

AU - Snoj, Luca

AU - Joyce, Malcolm

AU - Najdanovic‐Visak, Vesna

PY - 2023/12/13

Y1 - 2023/12/13

N2 - Despite offering low-carbon and reliable energy, the utilization of nuclear energy is declining globally due to high upfront capital costs and longer returns on investments. Nuclear cogeneration of valuable chemicals from waste biomass-derived feedstocks could have beneficial impacts while harnessing the underutilized resource of ionizing energy. Here, we demonstrate selective methanol or acetaldehyde production from ethylene glycol, a feedstock derived from glycerol, a byproduct of biodiesel, using irradiations from a nuclear fission reactor. The influence of radiation quality, dose rate, and the absorbed dose of irradiations on radiochemical yields (G-value) has been studied. Under low-dose-rate, γ-only radiolysis during reactor shutdown rate (

AB - Despite offering low-carbon and reliable energy, the utilization of nuclear energy is declining globally due to high upfront capital costs and longer returns on investments. Nuclear cogeneration of valuable chemicals from waste biomass-derived feedstocks could have beneficial impacts while harnessing the underutilized resource of ionizing energy. Here, we demonstrate selective methanol or acetaldehyde production from ethylene glycol, a feedstock derived from glycerol, a byproduct of biodiesel, using irradiations from a nuclear fission reactor. The influence of radiation quality, dose rate, and the absorbed dose of irradiations on radiochemical yields (G-value) has been studied. Under low-dose-rate, γ-only radiolysis during reactor shutdown rate (

U2 - 10.1021/acs.iecr.3c03317

DO - 10.1021/acs.iecr.3c03317

M3 - Journal article

C2 - 38107750

VL - 62

SP - 21152

EP - 21163

JO - Industrial and Engineering Chemistry Research

JF - Industrial and Engineering Chemistry Research

SN - 0888-5885

IS - 49

ER -