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Research output: Contribution to Journal/Magazine › Journal article › peer-review
Research output: Contribution to Journal/Magazine › Journal article › peer-review
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TY - JOUR
T1 - Breaking of valley degeneracy by magnetic field in monolayer MoSe2
AU - MacNeill, David
AU - Heikes, Colin
AU - Mak, Kin Fai
AU - Anderson, Zachary
AU - Kormanyos, Andor
AU - Zolyomi, Viktor
AU - Park, Jiwoong
AU - Ralph, Daniel C.
N1 - © 2015 American Physical Society
PY - 2015/1/22
Y1 - 2015/1/22
N2 - Using polarization-resolved photoluminescence spectroscopy, we investigate the breaking of valley degeneracy by an out-of-plane magnetic field in back-gated monolayer MoSe2 devices. We observe a linear splitting of -0.22 meV/T between luminescence peak energies in sigma(+) and sigma(-) emission for both neutral and charged excitons. The optical selection rules of monolayer MoSe2 couple the photon handedness to the exciton valley degree of freedom; so this splitting demonstrates valley degeneracy breaking. In addition, we find that the luminescence handedness can be controlled with a magnetic field to a degree that depends on the back-gate voltage. An applied magnetic field, therefore, provides effective strategies for control over the valley degree of freedom.
AB - Using polarization-resolved photoluminescence spectroscopy, we investigate the breaking of valley degeneracy by an out-of-plane magnetic field in back-gated monolayer MoSe2 devices. We observe a linear splitting of -0.22 meV/T between luminescence peak energies in sigma(+) and sigma(-) emission for both neutral and charged excitons. The optical selection rules of monolayer MoSe2 couple the photon handedness to the exciton valley degree of freedom; so this splitting demonstrates valley degeneracy breaking. In addition, we find that the luminescence handedness can be controlled with a magnetic field to a degree that depends on the back-gate voltage. An applied magnetic field, therefore, provides effective strategies for control over the valley degree of freedom.
KW - SPIN-LATTICE RELAXATION
KW - QUANTUM-WELLS
KW - DIAMAGNETIC SHIFT
KW - EXCITONS
KW - CDTE
KW - POLARIZATION
KW - TRANSITION
KW - ELECTRONS
U2 - 10.1103/PhysRevLett.114.037401
DO - 10.1103/PhysRevLett.114.037401
M3 - Journal article
VL - 114
JO - Physical review letters
JF - Physical review letters
SN - 0031-9007
IS - 3
M1 - 037401
ER -